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These are what almost made my Top 10, but are still some of the most enjoyable and/or interesting ones I've seen.

Honorable Favorites Rating
Air (TV) Good
Previously on my Top 10. Removed due to it's nature being unable to further compete with later replacements. Nonetheless, I love this series because of it's transitions, it's journey, it's ending, and the overall exp. Few series choose to do this, and such an impactful ending still has stayed with me, and doubtless ever will.
Air (movie) Decent
I love this movie more because it offers a pleasant "what if?" story than anything else. On it's own, and I haven't seen the TV series beforehand, this probably wouldn't be so high ranked.
Aura Battler Dunbine (TV) Good
While I haven't seen Ideon yet, I love this more than 1st Gundam. It's plot is more unpredictable, it's characters; more spacious with personality, and it's ending; more powerful. I call it one of Tomino's best.
Azumanga Daioh (TV) Excellent
Besides it being one of the easiest animes to rewatch and enjoy just as much as the first time around, it's mood and characters are such a joy to see again! It might be purer than most of it's kind, but in this case, it's vital.
Berserk (TV 1997) Masterpiece
I couldn't see the beauty of this show at first. It wasn't until it's 2nd half that I could see it's raw philosophical side, watch one of the best rising actions in anime, and see probably the most horrifying and disturbing endings I've ever seen. The very fact that I don't hate it because of that, only further convinces me of it's timelessness.
(The) Big O (TV) Very good
Just a very fun show with a not too often used plot theme added. It's mecha fights are some of the best I've seen, and the soundtrack; epic. To see a more thorough ending is a dream within dream, but it's always nice to see R. Dorothy every now and then.
Blue Gender (TV) Very good
The first mecha I watched AND finished. The slow, savory, moody style it uses to illustrate it's horrors is still something that shines within me. It's plot turned out to be a little underexposed, and turned the show into having a bit of a pacifistic message when it didn't really fit. Despite that, it still had plenty of resolving aspects, and one of it's core plots was handled nicely. I may give this series much more credit than it should now that I've seen more diverse titles, but it still holds the same amount of respect as when I watched it.
Brigadoon (TV) Very good
Casshern Sins (TV) Very good
Den-noh Coil (TV) Excellent
Dragon Ball Z: Cooler's Revenge (movie 5)
Evangelion: 2.0 You Can (Not) Advance (movie) Excellent
Future Boy Conan (TV) Excellent
Gankutsuou: The Count of Monte Cristo (TV) Excellent
Gravion (TV) Good
Infinite Ryvius (TV) Very good
Katanagatari (TV) Very good
Kaze no Stigma (TV) Decent
Kodocha (TV) Very good
(The) Legend of the Galactic Heroes (OAV) Masterpiece
Living for the Day After Tomorrow (TV) Very good
Marmalade Boy (TV) Very good
Moribito - Guardian of the Spirit (TV) Excellent
Mushi-Shi (TV) Excellent
My Neighbor Totoro (movie) Excellent
Neon Genesis Evangelion: The End of Evangelion (movie) Masterpiece
Nobody's Boy Remi (TV) Very good
Oh! Edo Rocket (TV) Very good
Only Yesterday (movie) Very good
Panty & Stocking with Garterbelt (TV) Very good
Persona 4: The Animation (TV) Very good
Planetes (TV) Masterpiece
Princess Tutu (TV) Masterpiece
Royal Space Force - The Wings of Honnêamise (movie) Excellent
Samurai 7 (TV) Good
School Rumble (TV) Very good
(The) Sky Crawlers (movie) Very good
Speed Grapher (TV) Very good
(The) Super Dimension Fortress Macross (TV) Excellent
(The) Super Dimension Fortress Macross: Do You Remember Love? (movie) Excellent
Turn A Gundam (TV) Excellent